3.11.68: All My Loving (BBC-2) 

Billed as a "film of pop music", Tony Palmer's "All My Loving" featured everyone
under the sun, including the Who, Beatles, Hendrix and Zappa. Pink Floyd's segment
had them performing a three-minute "Set The Controls" in an eerie setting of a
church -- extracts from which have been used by the BBC on many occasions since.
The entire show was last repeated in 1977, while the Floyd sequences were included
in Show 10 of "Sound of The 60's" in 1991. 

(from http://www4.pf-roio.de/pffan/voio/TV.html)

There are segments of these songs in the fim:

Cream - I Am So Glad
Cream - Toad
Pink Floyd - Set The Controls ..
The Who - Mary Ann With Shaky Hands
The Who - I Can See For Miles
The Who - My Generation
Donovan - The Lullaby Of Spring
The Animals - Good Times
Cream - We Are Going Wrong